Generating functions of the sequences $\binom{2n}{n}^2H_n$ and $\binom{2n}{n}^2H_{2n}$, where $H_n$ is $n$-th harmonic number, are known in terms of elliptic integrals $$ \sum_{n=1}^\infty\binom{2n}{n}^2\frac{H_n}{16^n}k^{2n}=K(\sqrt{1-k^2})+\frac{1}{\pi}K(k)\log\frac{k^2}{16(1-k^2)},\tag{1} $$ $$ \sum_{n=1}^\infty\binom{2n}{n}^2\frac{H_{2n}}{16^n}k^{2n}=\frac12K(\sqrt{1-k^2})+\frac{1}{\pi}K(k)\log\frac{k}{4(1-k^2)}.\tag{2} $$ Clausen's formula written in the form $$ \left[{}_2F_1\left({2a,2b\atop a+b+\tfrac12};x\right)\right]^2={}_3F_2\left({2a,~2b,~a+b\atop a+b+\tfrac12,2a+2b};4x(1-x)\right)\tag{3} $$ allows one to find the generating function of the sequence $\binom{2n}{n}^3(H_{2n}-H_n)$ by differentiating $(3)$ with respect to $a$ at $a=b=\tfrac14$: $$ \sum_{n=1}^\infty \binom{2n}{n}^3\frac{H_{2n}-H_n}{64^n}(4x(1-x))^n=\frac{2}{3\pi}K(\sqrt{x})\sum_{n=1}^\infty \binom{2n}{n}^2\frac{4H_{2n}-3H_n}{16^n}x^n.\tag{4} $$ Thus according to $(1)$ and $(2)$ this gf is known in terms of elliptic integrals.
Q: What can be said about the generating functions $\displaystyle f(x)=\sum_{n=1}^\infty \binom{2n}{n}^3\frac{H_n}{64^n}x^n$ and $\displaystyle g(x)=\sum_{n=1}^\infty \binom{2n}{n}^3\frac{H_{2n}}{64^n}x^n$ of the sequences $\binom{2n}{n}^3H_n$ and $\binom{2n}{n}^3H_{2n}$ separately?
In view of $(4)$ one can find closed form of $f(1)-g(1)$ and Whipple's sum http://dlmf.nist.gov/16.4.E7 (after differentiating it wrt $c$ at $a=c=\tfrac12,~d=1$) gives closed form of $2g(1)-3f(1)$. This means that at least the closed forms of $f(1)$ and $g(1)$ can be found.